1. Four Heavenly Kings
2. Stardust Crusaders
Man this arc is much more tense and emotional than in the manga, I just love it. This also made me wonder what exactly Polnareff use to do before going on this adventure.
2. Front Six
Nominating the Pillar Men- Jojo's Bizarre Adventure
I'll second the Bishokukai and the Saints
@Dream: He is referring to the the protagonist group of Part 3.